Great thread, spiggie.
It's worth noting that http://www.greatgifts.org is run by World Vision. Not that there's anything wrong with that; it's just that I personally wouldn't contribute to a Christian organisation like this.
Another option would be http://www.goodgifts.org, which has lots of participating charities. This one does have a compulsory handling charge of £4.95 though, which isn't great value if you're buying a Music Workshop for £12. The handling charge is used for sending a gift card to your recipient.
http://www.oxfamunwrapped.com is another alternative. I think Oxfam's version was set up quite recently. The other two sites have been established for quite a while now.
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